Napstablook's theme from Undertale. Given its whimsical nature, this track primarily fits lively sections such as bosses, athletic/auto-scrolling levels and bonus stages set in a haunted environment.
I agree with UTF on his 0:36 observation. On looking at the text file there is an ADSR command which makes the f^ note slightly sharper on channel #6 (zero indexed). Commenting out this command ($EE $60) makes it sound slightly better.
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